KR102716854B1 - Preparing method of high strength ceramic liquid absorber - Google Patents

Preparing method of high strength ceramic liquid absorber Download PDF

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KR102716854B1
KR102716854B1 KR1020220104007A KR20220104007A KR102716854B1 KR 102716854 B1 KR102716854 B1 KR 102716854B1 KR 1020220104007 A KR1020220104007 A KR 1020220104007A KR 20220104007 A KR20220104007 A KR 20220104007A KR 102716854 B1 KR102716854 B1 KR 102716854B1
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KR20240025859A (en
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강승진
정옥근
김동현
성동민
최봉석
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주식회사 이엠텍
주식회사 자이언트케미칼
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Priority to CN202380045063.6A priority patent/CN119546385A/en
Priority to PCT/KR2023/001414 priority patent/WO2024038985A1/en
Priority to JP2025505963A priority patent/JP2025525192A/en
Priority to EP23854959.6A priority patent/EP4574253A1/en
Priority to KR1020230108992A priority patent/KR20240026115A/en
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Abstract

실시예는 고강도 세라믹 흡습체의 제조 방법에 관한 것이다.
실시예는 금속 이온과 결합된 실리케이트 분말과 저온 소성용 글래스 분말을 혼합하는 제1 단계; 혼합 분말에 고분자 폴리머 및 분산제를 첨가하고 세라믹 과립을 제조하는 제2 단계; 세라믹 과립을 가압 성형하는 제3 단계; 및 성형체를 소결하는 제4 단계;를 포함하는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.
The invention relates to a method for manufacturing a high-strength ceramic moisture absorbent.
The invention provides a method for producing a high-strength ceramic moisture absorbent, comprising: a first step of mixing a silicate powder combined with metal ions and a glass powder for low-temperature firing; a second step of adding a high molecular polymer and a dispersant to the mixed powder and producing ceramic granules; a third step of pressurizing and molding the ceramic granules; and a fourth step of sintering the molded body.

Description

고강도 세라믹 흡습체의 제조 방법{PREPARING METHOD OF HIGH STRENGTH CERAMIC LIQUID ABSORBER}{PREPARING METHOD OF HIGH STRENGTH CERAMIC LIQUID ABSORBER}

실시예는 고강도 세라믹 흡습체의 제조 방법에 관한 것이다. The invention relates to a method for manufacturing a high-strength ceramic moisture absorbent.

액상을 이용한 에어로졸발생장치가 개발되어 널리 이용되고 있다. Aerosol generating devices using liquids have been developed and are being widely used.

도 1은 종래 기술에 따른 액상을 기재로 사용하는 에어로졸발생장치를 도시한 것이다. Figure 1 illustrates an aerosol generating device using a liquid as a substrate according to conventional technology.

흡입로드(90)는 흡입통(1), 무화장치(2), 액상분리시트(31)와 액상 저장체(32)를 포함하는 액상 유도 어셈블리(3), 마우스피스 커버(4), 유도관(5) 및 장식 슬리브(6)를 포함한다.The suction rod (90) includes a suction tube (1), an atomizer (2), a liquid induction assembly (3) including a liquid separation sheet (31) and a liquid storage body (32), a mouthpiece cover (4), an induction tube (5), and a decorative sleeve (6).

상기 흡입통(1)은 상기 무화장치(2), 액상유도 어셈블리(3), 마우스피스 커버(4) 및 유도관(5)을 설치하기 위한 것으로서, 흡입통(1)은 가운데가 통하는 원통체 구조이며, 본 실시예에서 이는 원통형 케이스로, 투명 또는 반투명 재질의 일자형 튜브재를 절단 가공하여 형성하였고, 흡입통(1)의 길이는 필요에 따라 튜브재를 필요한 길이로 절단하여 형성할 수 있다. 흡입통(1)은 말단 및 결합단부를 포함하며, 마우스피스 커버(4)는 사용자가 흡연할 수 있도록 상기 말단에 끼워지고, 결합단부는 배터리로드(미도시)와 서로 정합된다.The above-mentioned suction tube (1) is for installing the above-mentioned atomizer (2), a liquid induction assembly (3), a mouthpiece cover (4), and an induction tube (5), and the suction tube (1) has a cylindrical structure with an open center, and in this embodiment, it is a cylindrical case and is formed by cutting and processing a straight tube material made of a transparent or translucent material, and the length of the suction tube (1) can be formed by cutting the tube material to a required length as needed. The suction tube (1) includes a terminal end and a connecting end, and the mouthpiece cover (4) is fitted to the terminal end so that the user can smoke, and the connecting end is aligned with a battery load (not shown).

흡입통(1) 내부에 담배액상을 저장하기 위한 담배액상 탱크(11) 및 상기 전원로드(92)와 결합되기 위한 결합 어셈블리(12)가 더 설치되고, 상기 결합부재(12)는 무화장치(2)의 제1 전극(예를 들어 음전극)으로써의 제1 전극 부재(13)를 포함하며, 제1 전극부재(13)는 무화장치(2)의 제2 전극(예를 들어 양전극)으로써의 제2 전극부재 (14) 및 절연링(15)이 더 설치된다. 상기 담배액상 탱크(11)는 상기 흡입통(1) 내에 설치되며, 본 실시예에서 담배액상 탱크(11)는 상기 액상분리시트(31), 마우스피스 커버(4), 흡입통(1) 내벽 및 유도관(5) 외벽이 함께 한정하는 공간으로 형성되고, 액상분리시트(31) 및 마우스피스 커버(4)가 담배액상 탱크(11)의 양단을 밀봉함으로써 담배액상이 담배액상 탱크(11)에 밀봉된다.A tobacco liquid tank (11) for storing tobacco liquid inside the inhaler (1) and a coupling assembly (12) for coupling with the power load (92) are further installed, and the coupling member (12) includes a first electrode member (13) as a first electrode (e.g., a negative electrode) of the atomizer (2), and the first electrode member (13) is further provided with a second electrode member (14) as a second electrode (e.g., a positive electrode) of the atomizer (2) and an insulating ring (15). The above-mentioned tobacco liquid tank (11) is installed in the above-mentioned suction tube (1), and in this embodiment, the tobacco liquid tank (11) is formed by a space defined by the liquid separation sheet (31), the mouthpiece cover (4), the inner wall of the suction tube (1), and the outer wall of the induction pipe (5), and the liquid separation sheet (31) and the mouthpiece cover (4) seal both ends of the tobacco liquid tank (11), thereby sealing the tobacco liquid in the tobacco liquid tank (11).

이때, 무화장치(2)에서 가열에 의해 무화된 미세입자는, 유도관(5)을 타고 흡입구가 형성된 마우스피스 커버(4)측으로 이동하면서 일부가 액화되어 액적이 발생할 수 있다. 이때, 사용자는 미세입자를 흡입하며, 액화된 액적을 함께 입으로 흡입함으로써, 불쾌감을 느낄 수 있다. At this time, the fine particles that have been atomized by heating in the atomizer (2) may liquefy some of them and generate droplets as they move through the induction tube (5) toward the mouthpiece cover (4) where the suction port is formed. At this time, the user may feel discomfort by inhaling the fine particles and also inhaling the liquefied droplets into the mouth.

이를 개선하기 위해, 출원인은 기류 패스 관로 내에 외기와 액상이 지나갈 수 있는 기류 홀을 구비하는 다공성 흡습체를 배치하는 구조를 제안한 바 있다. To improve this, the applicant has proposed a structure in which a porous absorbent having airflow holes through which outside air and liquid can pass is placed within an airflow passage.

대한민국 등록특허 제10-2017920호Republic of Korea Patent No. 10-2017920

실시예는 고강도 세라믹 흡습체의 제조 방법을 제공하는 것을 목적으로 한다. The invention aims to provide a method for manufacturing a high-strength ceramic absorbent.

실시예는 금속 이온과 결합된 실리케이트 분말과 저온 소성용 글래스 분말을 혼합하는 제1 단계; 혼합 분말에 고분자 폴리머 및 분산제를 첨가하고 세라믹 과립을 제조하는 제2 단계; 세라믹 과립을 가압 성형하는 제3 단계; 및 성형체를 소결하는 제4 단계;를 포함하는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.The invention provides a method for producing a high-strength ceramic moisture absorbent, comprising: a first step of mixing a silicate powder combined with metal ions and a glass powder for low-temperature firing; a second step of adding a high molecular polymer and a dispersant to the mixed powder and producing ceramic granules; a third step of pressurizing and molding the ceramic granules; and a fourth step of sintering the molded body.

실시예의 다른 일 태양으로서, 실리케이트 분말은 Mg, Al, Zr, Li, Ba, MgAl, Na 및 Ca 중에서 선택된 하나 이상의 금속 이온을 포함하는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the silicate powder includes one or more metal ions selected from Mg, Al, Zr, Li, Ba, MgAl, Na and Ca.

실시예의 다른 일 태양으로서, 금속 이온과 결합된 실리케이트 분말은 BET법으로 측정된 비표면적이 20 내지 500m2/g인 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, wherein a silicate powder combined with a metal ion has a specific surface area of 20 to 500 m 2 /g as measured by the BET method.

실시예의 다른 일 태양으로서, 금속 이온과 결합된 실리케이트 분말의 평균 입경은 5 ~ 500㎛인 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the average particle size of the silicate powder combined with the metal ion is 5 to 500 ㎛.

실시예의 다른 일 태양으로서, 저온 소성용 글래스 분말은 아몰포스 글래스 분말 및 저온 소성용 세라믹 분말(Bi2O3, Sb2O5와 같은) 중 선택된 어느 하나 이상인 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the low-temperature firing glass powder is at least one selected from an amorphous glass powder and a low-temperature firing ceramic powder (such as Bi 2 O 3 and Sb 2 O 5 ).

실시예의 다른 일 태양으로서, 저온 소성용 글래스 분말은, 판상형, 파이버형, 다각형 중 어느 한 형태를 가지는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the glass powder for low-temperature firing has one of a plate shape, a fiber shape, and a polygonal shape.

실시예의 다른 일 태양으로서, 저온 소성용 글래스 분말은 600∼1200℃의 적정 소성 온도 범위를 가지는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the glass powder for low-temperature firing has an appropriate firing temperature range of 600 to 1200°C.

실시예의 다른 일 태양으로서, 저온 소성용 글래스 분말의 평균 입경은 0.5∼50㎛인 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for manufacturing a high-strength ceramic moisture absorbent is provided, characterized in that the average particle size of the low-temperature firing glass powder is 0.5 to 50 ㎛.

실시예의 다른 일 태양으로서, 저온 소성용 글래스 분말은 금속 이온과 결합된 실리케이트 분말 100 중량부 대비 1 중량부 내지 500 중량부 혼합되는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that a glass powder for low-temperature firing is mixed in an amount of 1 to 500 parts by weight relative to 100 parts by weight of a silicate powder combined with metal ions.

실시예의 다른 일 태양으로서, 제2 단계에서 첨가되는 고분자 폴리머는, 폴리비닐알콜, 폴리비닐 아세테이트, 폴리에틸렌, 폴리비닐부티렌, 폴리프로필렌, 폴리염화비닐, 폴리 아크릴, 폴리 아크릴 아미드, 구아 검, 젤라틴 및 천연고무 중에서 선택된 하나 이상의 물질인 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the high molecular weight polymer added in the second step is at least one material selected from polyvinyl alcohol, polyvinyl acetate, polyethylene, polyvinyl butylene, polypropylene, polyvinyl chloride, polyacrylic, polyacrylamide, guar gum, gelatin, and natural rubber.

실시예의 다른 일 태양으로서, 제2 단계에서 첨가되는 분산제는 습윤성 분산제인 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the dispersant added in the second step is a wettable dispersant.

실시예의 다른 일 태양으로서, 제2 단계에서 제조되는 세라믹 과립의 평균 입경은 50∼1000㎛인 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for producing a high-strength ceramic moisture absorbent is provided, characterized in that the average particle size of the ceramic granules produced in the second step is 50 to 1000 ㎛.

실시예의 다른 일 태양으로서, 제4단계의 소결은 600∼1200℃ 온도 범위에서 이루어지는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for manufacturing a high-strength ceramic moisture absorbent is provided, characterized in that the sintering in the fourth step is performed in a temperature range of 600 to 1200°C.

실시예의 다른 일 태양으로서, 제4단계의 소결 과정에서, 저온 소성용 글래스 분말의 표면 용융 및 넥킹 현상에 의해 세라믹 코어쉘 구조가 형성되는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법을 제공한다.As another aspect of the present invention, a method for manufacturing a high-strength ceramic moisture absorbent is provided, characterized in that a ceramic core-shell structure is formed by surface melting and necking of low-temperature sintering glass powder during the sintering process in the fourth step.

실시예가 제공하는 제조 방법을 통해 제조된 고강도 세라믹 흡습체는, 코어쉘 구조를 가져 고강도를 가진다는 장점이 있다. The high-strength ceramic moisture absorbent manufactured through the manufacturing method provided by the example has the advantage of high strength due to its core-shell structure.

도 1은 종래 기술에 따른 에어로졸 발생장치의 기화부를 상부에서 바라본 도면,
도 2는 실시예에 따른 고강도 세라믹 흡습체의 제조 방법의 플로우 차트,
도 3은 실시예에 따른 고강도 세라믹 흡습체의 제조 방법에 따라 제조된 세라믹 코어쉘 구조체의 개략도,
도 4는 실시예에 따른 고강도 세라믹 흡습체의 제조 방법에 따라 제조된 세라믹 코어쉘 구조체의 주사현미경 사진.
Figure 1 is a drawing of the vaporization part of an aerosol generator according to the prior art viewed from above.
Figure 2 is a flow chart of a method for manufacturing a high-strength ceramic moisture absorbent according to an embodiment.
Figure 3 is a schematic diagram of a ceramic core-shell structure manufactured according to a method for manufacturing a high-strength ceramic moisture absorbent according to an embodiment.
FIG. 4 is a scanning electron microscope photograph of a ceramic core-shell structure manufactured according to a method for manufacturing a high-strength ceramic moisture absorbent according to an embodiment.

이하, 도면을 참조하여 발명을 더욱 상세하게 설명한다.Hereinafter, the invention will be described in more detail with reference to the drawings.

도 2는 실시예에 따른 고강도 세라믹 흡습체의 제조 방법을 도시한 플로우 차트, 도 3은 실시예에 따른 고강도 세라믹 흡습체의 제조 방법에 따라 제조된 고강도 세라믹 흡습체의 개략도, 도 4는 실시예에 따른 고강도 세라믹 흡습체의 제조 방법에 따라 제조된 고강도 세라믹 흡습체의 주사현미경 사진이다. FIG. 2 is a flow chart illustrating a method for manufacturing a high-strength ceramic moisture absorbent according to an embodiment, FIG. 3 is a schematic diagram of a high-strength ceramic moisture absorbent manufactured according to a method for manufacturing a high-strength ceramic moisture absorbent according to an embodiment, and FIG. 4 is a scanning electron microscope photograph of a high-strength ceramic moisture absorbent manufactured according to a method for manufacturing a high-strength ceramic moisture absorbent according to an embodiment.

실시예에 따른 고강도 세라믹 흡습체의 제조 방법은 금속 이온과 결합된 실리케이트 분말과 저온 소성용 글래스 분말을 혼합하는 제1 단계(S1), 혼합 분말에 고분자 폴리머 및 분산제를 첨가하고 세라믹 과립을 제조하는 제2 단계(S2), 세라믹 과립을 가압 성형하는 제3 단계(S3) 및 성형체를 소결하는 제4 단계(S4)를 포함한다.A method for manufacturing a high-strength ceramic moisture absorbent according to an embodiment includes a first step (S1) of mixing silicate powder combined with metal ions and glass powder for low-temperature firing, a second step (S2) of adding a high molecular polymer and a dispersant to the mixed powder and manufacturing ceramic granules, a third step (S3) of pressurizing and molding the ceramic granules, and a fourth step (S4) of sintering the molded body.

이때, 제1 단계에서 혼합되는 실리케이트 분말은 Mg, Al, Zr, Li, Ba, MgAl, Na 및 Ca 중에서 선택된 하나 이상의 금속 이온을 포함한다. 이때, 금속 이온과 결합된 실리케이트 분말은 BET법으로 측정된 비표면적이 100 내지 450m2/g인 것이 바람직하며, 금속 이온과 결합된 실리케이트 분말의 평균 입경은 5 ~ 500㎛인 것이 바람직하다. At this time, the silicate powder mixed in the first step includes one or more metal ions selected from Mg, Al, Zr, Li, Ba, MgAl, Na, and Ca. At this time, the silicate powder combined with the metal ion preferably has a specific surface area of 100 to 450 m 2 /g as measured by the BET method, and the average particle size of the silicate powder combined with the metal ion is preferably 5 to 500 ㎛.

또한 제1 단계에서 실리케이트 분말과 혼합되는 저온 소성용 글래스 분말은 아몰포스 글래스 분말 및 저온 소성용 세라믹 분말 중 선택된 어느 하나 이상인 것이 바람직하다. 이때 저온 소성용 세라믹 분말은 Bi2O3, Sb2O5 등이 포함된다. In addition, it is preferable that the low-temperature firing glass powder mixed with the silicate powder in the first step is at least one selected from amorphous glass powder and low-temperature firing ceramic powder. At this time, the low-temperature firing ceramic powder includes Bi 2 O 3 , Sb 2 O 5 , etc.

이때, 저온 소성용 글래스 분말은, 판상형, 파이버형, 다각형 중 어느 한 형태를 가질 수 있으며, 저온 소성용 글래스 분말은 600∼1200℃의 적정 소성 온도 범위를 가지는 것이 바람직하다. 또한, 저온 소성용 글래스 분말의 평균 입경은 0.5∼50㎛인 것이 바람직하다. 이때, 저온 소성용 글래스 분말은 금속 이온과 결합된 실리케이트 분말 100 중량부 대비 1 중량부 내지 500 중량부 혼합된다.At this time, the glass powder for low-temperature firing may have any one of a plate shape, a fiber shape, and a polygonal shape, and it is preferable that the glass powder for low-temperature firing have an appropriate firing temperature range of 600 to 1200°C. In addition, it is preferable that the average particle size of the glass powder for low-temperature firing is 0.5 to 50 μm. At this time, the glass powder for low-temperature firing is mixed in an amount of 1 to 500 parts by weight relative to 100 parts by weight of the silicate powder combined with the metal ion.

글래스 분말 첨가량(wt%)Glass powder addition amount (wt%) 하중(N)Load (N) 굽힘 강도(Mpa)Bending strength (Mpa) 11 1414 3.903.90 33 2424 6.056.05 3030 4545 8.818.81 5050 7878 9.989.98

표 1은 저온 소성용 글래스 분말 첨가량에 따른 굽힘 강도를 측정한 값을 정리한 표이다. 저온 소성용 글래스 분말 첨가량이 많아질수록 굽힘 강도가 증가하는 것을 알 수 있다. Table 1 shows the values of bending strength measured according to the amount of low-temperature firing glass powder added. It can be seen that the bending strength increases as the amount of low-temperature firing glass powder added increases.

한편, 제2 단계에서 첨가되는 고분자 폴리머는, 폴리비닐알콜, 폴리비닐 아세테이트, 폴리에틸렌, 폴리비닐부티렌, 폴리프로필렌, 폴리염화비닐, 폴리 아크릴, 폴리 아크릴 아미드, 구아 검, 젤라틴 및 천연고무 중에서 선택된 하나 이상의 물질인 것이 바람직하며, 분산제는 습윤성 분산제인 것이 바람직하다. Meanwhile, the high molecular weight polymer added in the second step is preferably one or more substances selected from polyvinyl alcohol, polyvinyl acetate, polyethylene, polyvinyl butylene, polypropylene, polyvinyl chloride, polyacrylic, polyacrylamide, guar gum, gelatin, and natural rubber, and the dispersant is preferably a wetting dispersant.

제2 단계에서 제조되는 세라믹 과립의 평균 입경은 50∼1000㎛인 것이 바람직하다.It is preferable that the average particle size of the ceramic granules manufactured in the second step be 50 to 1000 μm.

한편, 제3 단계는, 세라믹 과립을 1축 또는 다축 가압하여 성형되며, 세라믹 흡습체를 원하는 형태로 압축 성형하는 단계이다. Meanwhile, the third step is a step of compressing and molding the ceramic absorbent into a desired shape by pressing the ceramic granules in one or multiple axes.

제4단계의 소결은 저온 소성용 글래스 분말의 적정 소성 온도에 맞추어 600∼1200℃ 온도 범위에서 이루어지는 것이 바람직하다. It is desirable that the sintering in the fourth stage be performed at a temperature range of 600 to 1200°C to match the appropriate sintering temperature of the glass powder for low-temperature sintering.

제4단계의 소결 과정을 거치면서,저온 소성용 글래스 분말의 표면 용융 및 넥킹 현상에 의해 세라믹 코어쉘 구조가 형성된다. 즉, 고강도 세라믹 흡습체는 1600℃ 이상의 고온 소성이 필요한 금속 이온과 결합된 실리케이트 분말에 저온 소성용 글래스 분말을 첨가함으로써, 상대적으로 낮은 600 ~ 1200℃의 온도에서 소결하여도 1Mpa 이상의 파괴 강도를 가진다는 장점이 있다. Through the sintering process of the fourth step, a ceramic core-shell structure is formed by the surface melting and necking phenomenon of the low-temperature sintering glass powder. That is, the high-strength ceramic moisture absorbent has the advantage of having a fracture strength of 1 MPa or more even when sintered at a relatively low temperature of 600 to 1200°C by adding low-temperature sintering glass powder to silicate powder combined with metal ions that require high-temperature sintering of 1600°C or higher.

한편, 실시예의 방법에 따라 제조된 고강도 세라믹 흡습체는, 에어로졸 발생장치에 설치되어 액상 흡수용으로 사용되거나, 담체용으로 사용될 수 있다. 또한 고강도를 유지하며 액체를 머금어야 하는 흡습체가 필요한 경우라면 어떠한 곳에든 적용할 수 있다. Meanwhile, the high-strength ceramic absorbent manufactured according to the method of the embodiment can be installed in an aerosol generating device and used for liquid absorption or as a carrier. In addition, it can be applied to any place where an absorbent that maintains high strength and can hold liquid is required.

Claims (15)

Mg, Al, Zr, Li, Ba, MgAl, Na 및 Ca 중에서 선택된 하나 이상의 금속 이온과 결합된 실리케이트 분말로, BET법으로 측정된 비표면적이 100 내지 450 m2/g이고 평균 입경은 5 ~ 500 ㎛인 금속 이온과 결합된 실리케이트 분말과, 아몰포스 글래스 분말 및 저온 소성용 세라믹 분말 중 선택된 어느 하나 이상인 0.5∼50 ㎛의 평균 입경을 갖고 Bi2O3, Sb2O5 중 어느 하나이고, 판상형, 파이버형, 다각형 중 어느 한 형태을 갖고 600∼1200 ℃의 적정 소성 온도 범위를 갖는 저온 소성용 글래스 분말을, 금속 이온과 결합된 실리케이트 분말 100 중량부 대비 1 중량부 내지 500 중량부의 저온 소성용 글래스 분말의 양으로 혼합하는 제1 단계;
혼합 분말에 폴리비닐알콜, 폴리비닐아세테이트, 폴리에틸렌, 폴리비닐부티렌, 폴리프로필렌, 폴리염화비닐, 폴리아크릴, 폴리아크릴아미드, 구아검, 젤라틴 및 천연고무 중에서 선택된 하나 이상의 물질인 고분자 폴리머 및 습윤성 분산제인 분산제를 첨가하여 50∼1000 ㎛의 평균 입경을 갖는 세라믹 과립을 제조하는 제2 단계;
세라믹 과립을 가압 성형하는 제3 단계;및
성형체를 600∼1200 ℃ 온도 범위에서 소결하는 제4 단계;를 포함하되,
제4 단계의 소결 과정에서, 저온 소성용 글래스 분말의 표면 용융 및 넥킹 현상에 의해 코어(110)의 표면에 저온 소성용 글래스 분말에 의한 쉘(120)이 형성되어 세라믹 코어쉘 구조를 갖는 다공성 구조체가 얻어지는 것을 특징으로 하는 고강도 세라믹 흡습체의 제조 방법.
A first step of mixing a silicate powder combined with at least one metal ion selected from Mg, Al, Zr, Li, Ba, MgAl, Na and Ca, the silicate powder having a specific surface area of 100 to 450 m2 /g as measured by the BET method and an average particle size of 5 to 500 ㎛, and a low-temperature firing glass powder having an average particle size of 0.5 to 50 ㎛, the glass powder having a shape of platelet, fiber or polygonal, and an appropriate firing temperature range of 600 to 1200° C , the glass powder having a shape of Bi2O3 or Sb2O5 and being at least one selected from amorphous glass powder and a low-temperature firing ceramic powder, the glass powder having a shape of platelet, fiber or polygonal, and an appropriate firing temperature range of 600 to 1200°C, in an amount of 1 part by weight to 500 parts by weight per 100 parts by weight of the silicate powder combined with the metal ion;
A second step of manufacturing ceramic granules having an average particle size of 50 to 1000 ㎛ by adding a polymer, which is at least one material selected from polyvinyl alcohol, polyvinylacetate, polyethylene, polyvinyl butylene, polypropylene, polyvinyl chloride, polyacryl, polyacrylamide, guar gum, gelatin, and natural rubber, and a dispersant, which is a wetting dispersant, to the mixed powder;
The third step of pressurizing and molding the ceramic granules; and
A fourth step of sintering the molded body at a temperature range of 600 to 1200 ℃; including;
A method for manufacturing a high-strength ceramic moisture absorbent, characterized in that, in the sintering process of the fourth step, a shell (120) made of low-temperature sintering glass powder is formed on the surface of the core (110) by surface melting and necking of the low-temperature sintering glass powder, thereby obtaining a porous structure having a ceramic core-shell structure.
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KR101989800B1 (en) 2017-08-08 2019-06-17 주식회사 테코플러스 antimicrobial and dehumidifying agent having deodorizing activity, method for manufacturing the same, and polyolefin film and laminated SHeet for shoes insole comprising the same
KR102039672B1 (en) 2015-07-10 2019-11-01 주식회사 엘지화학 Moisture absorption material for drying appaaratus

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KR102039672B1 (en) 2015-07-10 2019-11-01 주식회사 엘지화학 Moisture absorption material for drying appaaratus
KR101989800B1 (en) 2017-08-08 2019-06-17 주식회사 테코플러스 antimicrobial and dehumidifying agent having deodorizing activity, method for manufacturing the same, and polyolefin film and laminated SHeet for shoes insole comprising the same

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