CN101215301A - Full process cleaning production pollution prevention method for xylose and xylitol - Google Patents

Full process cleaning production pollution prevention method for xylose and xylitol Download PDF

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Publication number
CN101215301A
CN101215301A CNA2008100137121A CN200810013712A CN101215301A CN 101215301 A CN101215301 A CN 101215301A CN A2008100137121 A CNA2008100137121 A CN A2008100137121A CN 200810013712 A CN200810013712 A CN 200810013712A CN 101215301 A CN101215301 A CN 101215301A
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resin
liquid
concentration
wash
xylitol
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郑庆义
邵荣珠
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Abstract

The invention relates to a process for preventing pollution of xylose and xylitol total flow process cleaning production, which comprises the steps of water scouring, boiling, hydrolytic decomposition, filtering, ion exchange and condensation, wherein flushing cationic resin column and anion resin column with ionized water after finished ion exchange step to remove residual and disintegrated resin in resin layer, filtering out solid foreign substances in anion resin flushed solution and ion resin flushed solution through filtering process, detecting the concentration of metal salt in solution after removed solid foreign substances, respectively filling in HCL and NaOH and the concentration of HCL or NaOH reaches to 3-5% when the concentration of salt is lower or equal to 2%, and reusing cleaning solution after regulated to flush resin column, mixing anion resin flushed solution and ion resin flushed solution when the concentration is higher than 2%, desalting solution by desalting film, thereby obtaining strong brine and supernatant. Hazardous material such as waste water and waste slag which is generated in the production process of xylose and xylitol is completely eliminated through adopting the technical scheme, and the total flow process cleaning production is realized, therefore xylose production enterprises become environment-friendly enterprises.

Description

The method that wood sugar and the cleaner production of Xylitol whole process are prevented and remedied pollution
Technical field
The present invention relates to the method that a kind of wood sugar and the cleaner production of Xylitol whole process are prevented and remedied pollution.
Background technology
Wood sugar, formal name used at school five-carbon ring aldehydo sugar, profile is a white crystal, and its sugariness is equivalent to sucrose, and heat is lower than glucose, edible back cool taste.Xylitol is made by the wood sugar hydrogenation, is white crystal, and appearance is similar with sucrose, is sweeting agent the sweetest in the polyvalent alcohol, and flavor is cool, sugariness is equivalent to sucrose, and heat is equivalent to glucose.Being following sweeting agent, is sucrose and glucose substitute.Xylitol is a kind of sweet taste substance with nutritive value, also is the normal intermediate of human body sugar metabolism.At occurring in nature, Xylitol extensively is present in various fruit, the vegetables.The commodity Xylitol is with in the agricultural crops such as corn cob, bagasse, makes through deep processing, and be a kind of sweeting agent of natural health.At present, have severe contamination in the production process of wood sugar and Xylitol, mainly show following several respects: contained xylose solution fails to be used in hydrolysis residue and the hydrolysis residue, and the sepage stink is unpleasant in the air storage, and is seriously polluted; In and operation can produce a large amount of calcium sulfate, bleaching process produces a large amount of activity charcoal powders, these calcium sulfate and activity charcoal powder also can cause environmental pollution as processing and utilizing in addition not; Resin regeneration produces a large amount of HCL, NaOH, and multiple salts solution, will not cause water to pollute if do not add to handle to discharge; There are a large amount of impurity in the crystalline mother solution, are directly used in the quality that foodstuff production gently then reduces product as not removing, heavy then be detrimental to health.As application number is that 03110852.0 Chinese patent application " extracting the method for wood sugar and Xylitol from crop stalk " discloses a kind of to be raw material with the crop stalk, to produce the method for wood sugar and Xylitol through steps such as raw material pulverizing, washing, boiling, hydrolysis, filtration, ion-exchange, evaporation concentration, spraying dryings.Though this method is produced wood sugar and Xylitol has certain advance, the waste water, the waste residue that produce in producing have bigger contaminative to environment, can the serious harm environmental health as not handled.
Summary of the invention
The purpose of this invention is to provide and a kind ofly can overcome the wood sugar of above-mentioned pollution problem and the method that the cleaner production of Xylitol whole process is prevented and remedied pollution.
For achieving the above object, the present invention adopts following technical scheme:
The method that wood sugar of the present invention and the cleaner production of Xylitol whole process are prevented and remedied pollution, comprise raw material pulverizing, washing, boiling, hydrolysis, filtration, ion-exchange, concentrate each step, it is characterized in that: after ion-exchange step, wash cationic resin column and resin anion(R.A) post respectively with deionized water, remove foreign material and broken resin in the resin layer, obtain behind the positive resin wash liquid and negative resin respectively and wash back liquid; Filter out liquid and negative resin behind the positive resin wash respectively with filtering method and wash solid impurity in the liquid of back, remove after the solid impurity wherein, detect the wherein concentration of metal-salt, when the concentration of salt is less than or equal to 2%, add HCL in the liquid behind the resin wash on the sunny side, after negative resin is washed, add NaOH in the liquid, make the concentration of HCL or NaOH reach 3-5%, will adjust later washing lotion again and be used as the repeated use of flushing resin column; When the concentration of salt is higher than 2% in the liquid after liquid or negative resin behind the positive resin wash are washed, liquid and negative resin behind the positive resin wash are washed back liquid to be mixed, again through the desalination membrane desalination, obtain strong brine and clear liquid respectively, strong brine is used to evaporate salt manufacturing, clear liquid adds HCL or NaOH, is respectively applied for positive resin of flushing or negative resin.
At digestion process, be with 110-135 ℃ high-temperature water boiling 2 hours; The sulfuric acid concentration that uses in hydrolytic process is 0.5%-0.7%, and concentration of hydrochloric acid is 0.2-0.3%; At filtration step, adopt the three-stage filtration method, one-level is filtered 5-1 micron, cascade filtration 1-0.5 micron, three-stage filtration 0.01-0.001 micron.
Adopt this technical scheme, utterly destroyed the objectionable impurities of contaminate environment such as the waste water that produces in wood sugar and the Xylitol production process, waste residue, reach the standard of whole process cleaner production, make xylose production enterprise become environment-friendly type enterprise.
Embodiment
The method that wood sugar of the present invention and the cleaner production of Xylitol whole process are prevented and remedied pollution, with common production wood sugar and Xylitol process is prototype, processing parameter by reasonable each stage of adjustment also increases the regeneration of the ion exchange resin post after the ion-exchange and the harmless treatment of regenerated liquid, reach to reduce and pollute, so free of contamination purpose.It is as follows specifically to improve one's methods.
A) at washing, digestion process, adopt the method for hot-water extraction and washing, separation and Extraction comes out to be used to produce fertilizer with the raw material after pulverizing such as the submember in the corn cob--solid except that Mierocrystalline cellulose, xylogen, pentosan and liquid component--, avoids the residue contamination environment.Concrete grammar is, the processing of--immersion--stranding mill destroys cell walls with raw material pulverizing, makes raw material no longer contain liquid; Use 110-135 ℃ high-temperature water boiling 2 hours again, submember is separated, the method that washes with water is removed submember, obtains purified main component Mierocrystalline cellulose, xylogen and pentosan as hydrolysis material;
Can use one, two, three filtration method, filter step by step, reclaim submember, so both can guarantee the pure of filtrate, can avoid too big solid particulate to stop up filter screen again.Filtrate filtered is reused aborning, avoids the contaminated wastewater environment.
B) in hydrolytic process, adopt the low acid-hydrolysis method of high temperature.Specific practice is: improve hydrolysis temperature more than or equal to 110 ℃, between 110-135 ℃, be incubated 2 hours; Simultaneously, reduce acid concentration, use vitriolic concentration to be 0.5%-0.7%, the concentration of hydrochloric acid is 0.2-0.3%.The result who does like this is, hydrolyzed solution purity height, and it is low to contain acid concentration.Hydrolysis residue is purified corpus fibrosum and xylogen, can be used as the development of raw materials related products.Avoid depleted corpus fibrosum and xylogen contaminate environment.
C), the hydrolysis xylose solution is filtered purification through one, two, three at filtration step.One-level is filtered the 5-1 micron, cascade filtration 1-0.5 micron, and three-stage filtration 0.01-0.001 micron, like this, and can be with tiny solid substance, pigment is removed, and obtains the high xylose solution of purity level, and the solid substance that filtration is held back can be used to produce bio-feritlizer and be used.This step has been removed neutralized reaction product calcium sulfate in the old technology and decolouring its lytic activity carbon dust, has also reduced the loss of xylose solution.
D) in ion-exchange step
In wood sugar, the pure industry of wood sugar and other chemical industries, the technology of every use ion-exchange all can produce pollution in the resin regeneration process now, all must administer.Adopt positive resin and negative resin to adorn post respectively in the xylose production and carry out ion-exchange, in order to remove metal ion and the various acid group in the xylose solution.After ion-exchange, wash cationic resin column and resin anion(R.A) post respectively with deionized water, remove foreign material and broken resin in the resin layer, obtain behind the positive resin wash liquid and negative resin respectively and wash back liquid; Filter out liquid and negative resin behind the positive resin wash respectively with filtering method and wash solid impurity in the liquid of back, after removal solid wherein is assorted, detect the wherein concentration of metal-salt, when the concentration of salt is less than or equal to 2%, add HCL in the liquid behind the resin wash on the sunny side, after negative resin is washed, add NaOH in the liquid, make the concentration of HCL or NaOH reach 3-5%, will adjust later washing lotion again and be used as the repeated use of flushing resin column; When the concentration of salt is higher than 2% in the liquid after liquid or negative resin behind the positive resin wash are washed, liquid and negative resin behind the positive resin wash are washed back liquid to be mixed, again through the demoulding desalination, obtain strong brine and clear liquid respectively, strong brine is used to evaporate salt manufacturing, clear liquid adds HCL or NaOH, is respectively applied for positive resin of flushing or negative resin.So just can reuse the waste liquid that produces in the ion exchange process, avoid the discharging of waste liquid contaminate environment.
E) at enrichment step:
Maximum power consumption is 5% xylose solution in the xylose production, and reduction vaporization is concentrated into 35%.
Present method adopts cold concentration technology and equipment, promptly adopts reverse osmosis membrane that the hydrolysis xylose solution is concentrated into 40-50% by starting point concentration, greatly reduces to concentrate power consumption.
F) spraying drying, the cancellation mother liquor is received wood sugar entirely.
Old technology adopts evaporation concentration to xylose concentration 75%-80%, and crystalline xylose is extracted in crystallization, centrifugation, and the impurity major part is stayed in the mother liquor.Present method reaches 40-50% with cold concentration technology with xylose concentration, and spray-dried more full receipts wood sugar does not have mother liquor, and the prerequisite that adopts this method is the contaminant removal in the xylose solution, based on very high purity, and foreign matter content is lower than the finished product standard.Removal of contamination guarantees high purity, and this method is finished by two measures: the non-sugared impurity in the raw material is removed in high-temperature water extracting and washing; Remove neutralisation of sulphuric acid and decolouring activated carbon, stop to introduce tramp material in the technological process, cause foreign matter content extremely low.
So far, use this method raw material availability 100% in xylose production, do not have the discharging of residue solid substance.Waste liquids such as water, HCL, NaOH, NaCL are through purifying, and recycling does not have discharging.Realized the whole process cleaner production, really reached zero release, made xylose production enterprise become environment-friendly type enterprise.
The wood sugar hydrogenation can be produced Xylitol, and along with the realization of wood sugar prevention and cure of pollution, Xylitol is realized the whole process cleaner production equally.

Claims (2)

1. wood sugar and the cleaner production of the Xylitol whole process method of preventing and remedying pollution, comprise raw material pulverizing, washing, boiling, hydrolysis, filtration, ion-exchange, concentrate each step, it is characterized in that: after ion-exchange step, wash cationic resin column and resin anion(R.A) post respectively with deionized water, remove foreign material and broken resin in the resin layer, obtain behind the positive resin wash liquid and negative resin respectively and wash back liquid; Filter out liquid and negative resin behind the positive resin wash respectively with filtering method and wash solid impurity in the liquid of back, remove after the solid impurity wherein, detect the wherein concentration of metal-salt, when the concentration of salt is less than or equal to 2%, add HCL in the liquid behind the resin wash on the sunny side, after negative resin is washed, add NaOH in the liquid, make the concentration of HCL or NaOH reach 3-5%, will adjust later washing lotion again and be used as the repeated use of flushing resin column; When the concentration of salt is higher than 2% in the liquid after liquid or negative resin behind the positive resin wash are washed, liquid and negative resin behind the positive resin wash are washed back liquid to be mixed, again through the desalination membrane desalination, obtain strong brine and clear liquid respectively, strong brine is used to evaporate salt manufacturing, clear liquid adds HCL or NaOH, is respectively applied for positive resin of flushing or negative resin.
2. the method that wood sugar according to claim 1 and the cleaner production of Xylitol whole process are prevented and remedied pollution is characterized in that: at digestion process, be with 110-135 ℃ high-temperature water boiling 2 hours; The sulfuric acid concentration that uses in hydrolytic process is 0.5%-0.7%, and concentration of hydrochloric acid is 0.2-0.3%; At filtration step, adopt the three-stage filtration method, one-level is filtered 5-1 micron, cascade filtration 1-0.5 micron, three-stage filtration 0.01-0.001 micron.
CNA2008100137121A 2008-01-07 2008-01-07 Full process cleaning production pollution prevention method for xylose and xylitol Pending CN101215301A (en)

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Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN102703613A (en) * 2012-06-26 2012-10-03 山东福田药业有限公司 Xylose hydrolysate preparation pre-treatment method for papermaking wastewater
CN102839229A (en) * 2012-09-14 2012-12-26 武汉工程大学 Method for increasing reducing sugar yield by coupling of membrane separation and lignocellulose acid hydrolysis
CN116041405A (en) * 2022-12-29 2023-05-02 陕西科技大学 Method for separating sucrose-glucose-fructose in plants

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN102703613A (en) * 2012-06-26 2012-10-03 山东福田药业有限公司 Xylose hydrolysate preparation pre-treatment method for papermaking wastewater
CN102839229A (en) * 2012-09-14 2012-12-26 武汉工程大学 Method for increasing reducing sugar yield by coupling of membrane separation and lignocellulose acid hydrolysis
CN116041405A (en) * 2022-12-29 2023-05-02 陕西科技大学 Method for separating sucrose-glucose-fructose in plants

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Open date: 20080709