WO2008110113A1 - Multi-function health care self-cleaning shoe material - Google Patents

Multi-function health care self-cleaning shoe material Download PDF

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Publication number
WO2008110113A1
WO2008110113A1 PCT/CN2008/070464 CN2008070464W WO2008110113A1 WO 2008110113 A1 WO2008110113 A1 WO 2008110113A1 CN 2008070464 W CN2008070464 W CN 2008070464W WO 2008110113 A1 WO2008110113 A1 WO 2008110113A1
Authority
WO
WIPO (PCT)
Prior art keywords
shoe material
cleaning shoe
material according
fibers
functional health
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
PCT/CN2008/070464
Other languages
English (en)
French (fr)
Inventor
Hung-Jen Chen
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
U BOND Inc
Original Assignee
U BOND Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by U BOND Inc filed Critical U BOND Inc
Priority to NZ579521A priority Critical patent/NZ579521A/en
Priority to JP2009552995A priority patent/JP2010520792A/ja
Priority to AU2008226237A priority patent/AU2008226237B2/en
Priority to US12/449,891 priority patent/US20100050469A1/en
Priority to EP08715200A priority patent/EP2130448A4/en
Priority to MX2009009275A priority patent/MX2009009275A/es
Priority to CA002682318A priority patent/CA2682318A1/en
Publication of WO2008110113A1 publication Critical patent/WO2008110113A1/zh
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

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Classifications

    • A—HUMAN NECESSITIES
    • A43—FOOTWEAR
    • A43B—CHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B17/00—Insoles for insertion, e.g. footbeds or inlays, for attachment to the shoe after the upper has been joined
    • A43B17/10—Insoles for insertion, e.g. footbeds or inlays, for attachment to the shoe after the upper has been joined specially adapted for sweaty feet; waterproof
    • A43B17/102—Moisture absorbing socks; Moisture dissipating socks
    • A—HUMAN NECESSITIES
    • A43—FOOTWEAR
    • A43B—CHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B1/00—Footwear characterised by the material
    • A43B1/0009—Footwear characterised by the material made at least partially of alveolar or honeycomb material
    • A—HUMAN NECESSITIES
    • A43—FOOTWEAR
    • A43B—CHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B1/00—Footwear characterised by the material
    • A43B1/0045—Footwear characterised by the material made at least partially of deodorant means
    • A—HUMAN NECESSITIES
    • A43—FOOTWEAR
    • A43B—CHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B1/00—Footwear characterised by the material
    • A43B1/02—Footwear characterised by the material made of fibres or fabrics made therefrom
    • A43B1/05—Footwear characterised by the material made of fibres or fabrics made therefrom woven
    • A—HUMAN NECESSITIES
    • A43—FOOTWEAR
    • A43B—CHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B23/00—Uppers; Boot legs; Stiffeners; Other single parts of footwear
    • A43B23/02—Uppers; Boot legs
    • A43B23/0205—Uppers; Boot legs characterised by the material
    • A—HUMAN NECESSITIES
    • A43—FOOTWEAR
    • A43B—CHARACTERISTIC FEATURES OF FOOTWEAR; PARTS OF FOOTWEAR
    • A43B7/00—Footwear with health or hygienic arrangements
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T428/00—Stock material or miscellaneous articles
    • Y10T428/24—Structurally defined web or sheet [e.g., overall dimension, etc.]
    • Y10T428/24149—Honeycomb-like
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y10—TECHNICAL SUBJECTS COVERED BY FORMER USPC
    • Y10T—TECHNICAL SUBJECTS COVERED BY FORMER US CLASSIFICATION
    • Y10T428/00—Stock material or miscellaneous articles
    • Y10T428/24—Structurally defined web or sheet [e.g., overall dimension, etc.]
    • Y10T428/24777—Edge feature
    • Y10T428/24785—Edge feature including layer embodying mechanically interengaged strands, strand portions or strand-like strips [e.g., weave, knit, etc.]

Definitions

  • the present invention relates to a multifunctional functional health self-cleaning shoe material, which may be one of an upper, an insole or a sole. Background technique
  • shoes are essential for human daily life and most of the time. Wearing them for a long time every day has a great impact on health, especially the breathability and antibacterial efficacy of shoes.
  • the basic components of a typical shoe include a sole, a shoe upper, and an insole. As long as these members are designed to have breathability and antibacterial efficacy, the effectiveness of the shoe to ensure the health of the user can be surely improved.
  • the conventional structure is made of a non-woven fabric insole, and an antibacterial material is added to the non-woven fabric of the insole, which is not only insufficient in air permeability, easy to be worn, can not be easily cleaned for a long time, and has a short service life, and The insole cannot be effectively vibrated so that its functional substances cannot function in the foot environment.
  • a first object of the present invention is to provide a breathable effect of a shoe material having a better air permeability than a conventional product, and to form a good air cushion structure, and thereby reacting by the principle of frictional vibration between the foot and the fiber, air flow, cold and heat difference, etc.
  • Rice functional particles, multi-functional functional health self-cleaning shoes that achieve full and effective sterilization, antibacterial, anti-mildew, anti-mite, negative ion, far infrared, fire, anti-static, anti-electromagnetic wave and eliminate odor, TVOCs pollutants and other health and health effects material.
  • a second object of the present invention is to provide a multi-functional functional health self-cleaning shoe material which has the effects of long-lasting aromatherapy and the like.
  • a third object of the present invention is to provide a method for producing a multi-functional functional health self-cleaning shoe material.
  • the present invention adopts the following design scheme:
  • the multifunctional functional health self-cleaning shoe material of the invention adopts polypropylene or polyethylene chips and contains functional granular fibers (such as tourmaline, nano silver particles, enzymes, microcapsules and the like), and is kneaded. And melt-mixing and drawing the fiber to form a fiber mesh, and fabricating the fiber into a fabric mesh body, and designing the shoe material, such as an insole, a sole or a shoe upper, to make the shoe material have better ventilation effect than the conventional product, and Form a good steam cushion structure, and then through the friction between the foot and the fiber, the air flow, the difference between the cold and the heat and the weight of the human body to generate airflow to form the air cushion to absorb the functional particles of the nanometer, to achieve full and effective sterilization, antibacterial, anti-mildew, Anti-mite, negative ion, far infrared, fire, anti-static, anti-electromagnetic wave and eliminate odor, TVOCs, PMx pollutants and other health and health effects.
  • the multifunctional functional health self-cleaning shoe material of the invention is made of polypropylene or polyethylene chips, mixed and melted and mixed to form fibers and TPE controlled microcapsules to release and enhance resilience and comfort.
  • the microcapsules coated with natural extracting essential oil are mixed in the fiber, so that the shoe material has the effects of long-lasting aromatic health therapy.
  • Figure 1 is a perspective view of the shoe material of the present invention as an insole with shoes
  • Figure 2 is a plan view showing the shoe material of the present invention as an insole
  • Figure 3 is a schematic view of the shoe material of the present invention as an upper
  • Figure 4 is a partial cross-sectional view showing the fiber of the shoe material of the present invention
  • Figure 5 is a schematic view of another embodiment of the shoe material of the present invention.
  • Figure 6 is a schematic view showing an embodiment of the shoe material of the present invention with a cloth layer
  • Figure 7 is a schematic view showing an embodiment of the sole forming a slipper of the present invention
  • FIG. 8 is a schematic view showing the structure of the antenna body of the present invention having an array of stereo honeycomb structures
  • FIG. 9 is an enlarged schematic view of a three-dimensional honeycomb structure unit of the present invention.
  • Figure 10 is a side view of Figure 8.
  • Figure 11 is a schematic view of the upper mold and the first lower mold of the present invention
  • Figure 12 is a schematic view showing the molding process of the upper mold and the first lower mold according to the present invention
  • Figure 13 is a schematic view of the upper mold and the second lower mold of the present invention.
  • FIG. 14 is a schematic flow chart showing a molding process of an upper die and a second lower die according to the present invention.
  • the present invention mainly designs a multifunctional functional health self-cleaning shoe material, which may be one of an upper, an insole or a sole.
  • the basic structure includes a shoe body 10,
  • the shoe body 10 includes a peripheral contour area 11 and an inner circumference area 12; and a sheet-like net body 120 distributed in the inner circumference area 12 of the body 10, the net body 120 is fixed in the peripheral contour area 1 1
  • the mesh body 120 is a mesh-shaped braid comprising a plurality of warp fibers 13 and a plurality of weft fibers 13, and the fibers 13 are mixed with a plurality of functional particles 130 (please refer to FIG. 4). .
  • the main body of the fiber material may be a fiber having a wire diameter of 50-10000 denier and made of a material such as polypropylene, polyethylene, nylon or Tedron; and applied according to its characteristic requirements, for example, polypropylene can be resistant to strong acid and strong Alkali.
  • a plurality of reinforcing bodies 15 may be locally placed on the insole 100 or the sole 102.
  • the material of the reinforcing body 15 may be polyurethane (PU), thermoplastic elastomer (TPE, Thermoplastic Elastomer) or EPA, so that the effect is more enhanced.
  • Durability the method of directly injecting polyurethane (PU, Polyurethane), thermoplastic elastomer (TPE, Thermoplastic Elastomer) or EPA material into the insole 100 or the sole 102, after drying, can be formed on the insole 100 or the sole 102.
  • the shoe body 10 of the present invention may be a sole 102 (shown in FIG. 7) or an insole 100 (shown in FIGS. 1 and 2), or may be an upper 101 (shown in FIG. 3), wherein the insole 100 It is placed in the shoe 20 to space the sole and the sole of the person, thereby generating a cushioning air cushion and avoiding rapid wear of the sole.
  • the shoe body 10 is an insole 100, and the insole 100 includes the peripheral contour area 1 1 , the inner circumference area 12 and the net body 120.
  • the peripheral contour region 11 of the insole 100 can be a glue layer, and the end of the fiber 13 is fixed by the glue layer.
  • the shoe material is an insole 100
  • the peripheral contour area 1 1 of the insole 100 may also be a fusion line 1 10 that is thermally bonded to each other by the fibers 13 of the mesh body 120, and the fusion line 1 10 The end of the fiber 13 is fixed.
  • the shoe body 10 of the present invention when the shoe body 10 of the present invention is the sole 102 or the insole 100, it may include a plurality of layers of the woven mesh body 120, thereby increasing the thickness of the inner peripheral region 12, The air permeability and the cushioning air cushion performance are increased.
  • Each of the net bodies 120 is a mesh-like braid comprising a plurality of warp fibers 13 and a plurality of weft fibers 13, and the peripheral contour region 11 of each layer is a fiber. 13 A self-bonding fusion line 1 10, to which the ends of the fibers 13 are fixed. As shown in FIG.
  • the inner peripheral region 12 has at least one bonding portion 121 having a dot-like bonding portion or a line segment shape, and the bonding portion 121 is a mesh portion
  • the fibers 13 of the body 120 are self-bonded to each other, thereby improving the firmness of the overlapping of the respective mesh bodies 120.
  • the shoe body 10 of the present invention is an insole 100, which in turn may be designed to further include at least one cloth layer 14, which is covered on the net body 120 of the insole 100, and
  • the cloth layer 14 has a higher coefficient of friction than the net body 120.
  • the cloth layer 14 is bonded to the net body 120 of the insole 100 by at least one adhesive portion 140 in the form of a dot or a line segment, thereby improving the adhesion between the mesh body 120 and the cloth layer 14 .
  • the sole 102 is connected with a sleeve 103 which is curved and can be fitted over the foot of the human body to constitute a structural form of the slippers.
  • the mesh body 120 of the shoe material body of the present invention is woven to include a plurality of three-dimensional honeycomb structures 121 in an array, and each of the honeycomb structures 121 is composed of a plurality of the warp fibers. 13 is arranged along a first concave curved surface 122 and a plurality of the zonal fibers 13 are arranged along a second concave curved surface 123, wherein the first concave curved surface 122 and the second concave curved surface 123 are mutually cross.
  • the functional microparticles may be sub-micron tourmaline, so that the shoe material has the effects of generating negative ions, far infrared rays, self-cleaning, deodorizing, antistatic, anti-electromagnetic waves, and the like.
  • the functional particles may also be nano silver particles, so that the shoe material has the health functions of sterilization, antibacterial, anti-mildew, anti-mite, and may be added with chitin, enzyme or nano precious metal. Sterilization, antibacterial, antifungal factor of healthy microparticles of at least one of copper, zinc, gold, platinum, palladium, iridium and the like.
  • the functional microparticles may be microcapsules, and the microcapsules are internally provided with a receiving space filled with a layer of various functional materials, and the microcapsule shell material may be Chitosan, thermoplastic elastomer, etc., and this layer of functional material can be a natural essential oil to make the shoe have the function of long-lasting aromatic oil, and can be matched with lavender, lemon, eucalyptus, rosemary, and eucalyptus.
  • tea tree tea tree, sandalwood, bergamot, pine, jasmine, rose, chamomile, ylang ylang, basil, geranium, white layer, cardamom, musk, myrrh, cinnamon, anise, frankincense, orange, mint, cedar, patchouli Natural essential oil of at least one of rose grass, clove, grape sleeve, benzoin, ginger, lemongrass and marjoram.
  • the method for manufacturing a shoe material is to use at least one piece of mesh body 120, which comprises a plurality of warp fibers 13 and a plurality of weft fibers.
  • a mesh-like braid of 13 and the fiber 13 is internally mixed with a plurality of functional particles 130 (please refer to FIG. 4), and the mesh body 120 is provided with at least one fiber by ultrasonic processing.
  • 13 is fused to each other by a fusion line 110 (see FIG. 12), wherein the fusion line 110 is a peripheral contour area 11, and the network body 120 is separated by an inner circumference by the peripheral contour area 11.
  • Area 12, with the inner circumference area 12 as a shoe material The shape of the body 10.
  • the ultrasonic processing method includes an ultrasonic generating device 33, an upper mold 30, and a first lower mold 31, and the at least one The mesh body 120 is first placed between the upper die 30 and the first lower die 31, and the upper die 30 is clamped with the first lower die 31, and the upper die 30 is generated by the ultrasonic generating device 33.
  • the sound wave is vibrated, and the mesh body 120 is further provided with at least one fusion line 110 formed by the fibers 13 being fused to each other, and the fusion line 110 is the peripheral contour area 11 and the at least one is At least one of the inner peripheral regions 12 is partitioned from the mesh body 120, and then cut along the fusion line 110 by a cutting method to complete the manufacture of the shoe material.
  • the first lower die 31 is provided with at least one convex portion 310 in the shape of a dot or a line segment, and the at least one mesh body 120 is a phase.
  • the plurality of stacked net bodies 120 are formed in the inner peripheral region 12 of the plurality of net bodies 120 by a convex portion 310 to form a dot-shaped or line-shaped bonding portion 121.
  • the bonding portion 121 is a plurality of the bonding portions 121.
  • the fibers 13 of the net body 120 are bonded to each other.
  • the cutting method may further include a second lower mold 32, and the second lower mold 32 is provided with the fusion line 110.
  • a cutter 320 having a similar contour shape the mesh body 120 is placed between the upper mold 30 and the second lower mold 32, and the upper mold 30 and the second lower mold 32 are clamped by the ultrasonic generating device.
  • the upper mold 30 is subjected to ultrasonic vibration, and the cutter 320 of the second lower mold 32 is cut along the fusion line 110.
  • test conditions were humidity 58 %, temperature 29 ° C, and good fastness was maintained before and after the test, and the amount of negative ions generated was not reduced by washing.
  • the shoe material of the present invention is used to measure the concentration of ammonia (NH 3 ) and acetaldehyde (CH 3 CHO ) according to the JEM 1467 test method, and then the concentration of acetic acid (CH 3 COOH) is eliminated.
  • NH 3 ammonia
  • CH 3 CHO acetaldehyde
  • CH 3 COOH acetic acid
  • Table 5 Deodorization results of the shoe material of the present invention measured according to the JEM 1467 test method
  • Staphylococcus aureus 1.0 X 10' 3.0 x 10 4 99.9 (%) Escherichia coli 2.1 X 10' 1.6 x 10 3 99.9 (%) Klebsiella pneumoniae 7.3 X 10 5 3.0 x 10 4 95.9 (%)
  • Table 13 The results of Table 13 were obtained in accordance with the JEM 1467 test method for measuring the elimination efficiency of indoor air quality (IAQ).
  • the air quality (IAQ) of the present invention was found to have a long-lasting automatic cleaning ability as shown in Table 13 below.
  • Test item Test item Unit Test method Method detection ROHS limit Limit value NO.l
  • the fiber material of the shoe material of the invention is mixed with functional particles, so that the shoe material has functional properties such as sterilization, antibacterial, anti-mildew, anti-mite, negative ion, far infrared ray, fireproof, antistatic, anti-electromagnetic wave and odor elimination, TVOCs Health effects such as PMx and other pollutants.
  • the shoe material of the invention has a multi-layer structure for the insole, so that the fiber has better elasticity under the principle of balancing mechanical properties, and the fluid can pass through the shoe material to generate appropriate vibration performance, and the function in the fiber is stimulated.
  • Sexual particles are more active, and they achieve a functional cushion that effectively exerts its health function and enables the foot to be properly relieved and cushioned.
  • the shoe material of the present invention is an insole which is woven with fiber, has better ventilation, can achieve sanitary and health benefits and can be washed.
  • the shoe material of the present invention is added with functional particles (e.g., sub-micron tourmaline particles), and the mechanical strength of the shoe material produced by the invention is only slightly reduced, but does not have much influence.
  • functional particles e.g., sub-micron tourmaline particles
  • the sub-micron tourmaline particles of the present invention can effectively increase the lifting efficiency under the "electrostatic adsorption principle" due to the negative electric effect of the tourmaline, and the shoe material not only has better elasticity and friction, but also has special effects of negative ions - thermoelectricity, Under the piezoelectric accelerated water-decomposing anion (H 3 O 2 — ), the elastic vibration frequency is high and the friction is large. In the dynamic mode, a large amount of negative ions can be released, which can meet the human health demand (1000-2000ion). /cc) o
  • the essential oil is prevented from being quickly volatilized, and the essential oil can be released in a near quantitative manner to avoid waste and improve durability.
  • the shoe material of the present invention has a certain antibacterial effect.
  • the shoe material of the present invention also has a fireproof function, and can ensure absolute fire safety for use.

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Health & Medical Sciences (AREA)
  • Epidemiology (AREA)
  • General Health & Medical Sciences (AREA)
  • Public Health (AREA)
  • Footwear And Its Accessory, Manufacturing Method And Apparatuses (AREA)
  • Laminated Bodies (AREA)

Description

多功能机能性健康养生自净鞋材
技术领域
本发明涉及一种多功能机能性健康养生自净鞋材， 该鞋材可为鞋面、 鞋垫或 鞋底其中一种。 背景技术
目前鞋子为人类每日生活且大部份时间使用的必需品， 每日长时间穿著， 对 于身体健康的影响很大， 尤其是鞋子的透气性及抗菌效能相当重要。 一般鞋子的 组成基本构件包括有鞋底、 鞋面及鞋垫， 只要将这些构件设计成具有透气性及抗 菌效能， 便可确实提升鞋子确保使用者身体健康的效能。 目前所见到的惯用具有 抗菌功能的鞋材， 只有鞋垫具有抗菌功能， 鞋面及鞋底发明人等尚未有所见， 而 惯用的鞋垫结构， 虽皆强调为具有抗菌能力。 然而惯用结构， 都是以不织布制成 鞋垫， 再于鞋垫的不织布材添加抗菌的物质， 其不仅透气性不足， 穿著易有不适 感， 无法经简单清洗做长时间重复使用， 使用寿命短， 而且无法让鞋垫产生有效 的振动， 以致其机能性物质无法在足部环境中发挥其作用。 发明内容
本发明的第一目的是提供一种可使鞋材较传统产品具有更佳的透气效果， 并 形成良好气垫结构， 进而通过足部与纤维间摩擦震动、 空气流动、 冷热差等原理 反应奈米机能性粒子， 达到充分有效杀菌、 抗菌、 防霉、 防螨、 负离子、 远红外 线、 防火、 抗静电、 抗电磁波及排除异味、 TVOCs 污染物等健康养生功效的多 功能机能性健康养生自净鞋材。
本发明的第二目的在于提供一种使鞋材具有持久芳香养生疗法等功效的多 功能机能性健康养生自净鞋材。
本发明的第三目的在于提供一种具有多功能机能性健康养生自净鞋材的制 造方法。
为实现上述目的， 本发明采取以下设计方案：
本发明的有益效果是：
1、 本发明多功能机能性健康养生自净鞋材， 其采用聚丙烯或聚乙烯碎片内 混含有机能性微粒纤维 （如电气石、 奈米银粒子、 酵素、 微胶囊等微粒） ， 混练 及熔融混合抽丝而制成纤维， 以该纤维织制成织物网体， 并设计制作成鞋材， 如 鞋垫、 鞋底或鞋面， 可使鞋材较传统产品具有更佳的透气效果， 并形成良好汽垫 结构， 进而通过足部与纤维间摩擦震动、 空气流动、 冷热差及人体运动重量产生 气流形成气垫呼吸等原理反应奈米机能性粒子，达到充分有效杀菌、抗菌、防霉、 防螨、 负离子、 远红外线、 防火、 抗静电、 抗电磁波及排除异味、 TVOCs、 PMx 污染物等健康养生功效。
2、 本发明多功能机能性健康养生自净鞋材， 采用聚丙烯或聚乙烯碎片内混 含有， 混练及熔融混合抽丝而制成纤维及 TPE 控制微胶囊释放及增强回弹性及 舒适度， 并于纤维内混掺包覆有天然萃取精油的微胶囊， 因此使鞋材具有持久芳 香养生疗法等功效。 附图说明
图 1为本发明鞋材为鞋垫搭配鞋子的立体示意图
图 2为本发明鞋材为鞋垫的平面示意图
图 3为本发明鞋材为鞋面的示意图
图 4为本发明鞋材的纤维的局部断面示意图
图 5为本发明鞋材的另一实施例示意图
图 6为本发明鞋材加设有布层的实施例示意图
图 7为本发明鞋底形成拖鞋的实施例示意图
图 8为本发明网体具有阵列立体蜂巢结构示意图
图 9为本发明立体蜂巢结构单元放大示意图
图 10为图 8的侧面示意图
图 11为本发明上模与第一下模示意图
图 12为本发明上模与第一下模合模成型流程示意图
图 13为本发明上模与第二下模示意图
图 14为本发明上模与第二下模合模成型流程示意图 具体实施方式
为便于进一步了解本发明的目的手段， 兹附以较佳实施例图详细说明如后： I .本发明的鞋材基本构造
请参看图 1所示， 本发明主要在设计一种多功能机能性健康养生自净鞋材， 该鞋材可以是鞋面、 鞋垫或鞋底其中一种。 其基本结构包括有一鞋材本体 10， 该 鞋材本体 10包括有周边轮廓区域 1 1及内围区域 12; 以及一分布在该本体 10的 该内围区域 12的片状网体 120， 该网体 120被固定在该周边轮廓区 1 1上， 该网 体 120为包括有复数条经向纤维 13及复数条纬向纤维 13的网状编织体， 而且该 纤维 13内混含有复数个机能性微粒 130(请配合参看图 4所示)。 纤维材料主体可 为线径为 50- 10000丹尼， 并以聚丙烯、 聚乙烯、 尼龙或特多龙等材料制成的纤 维； 依其特性需求来加以应用， 例如聚丙烯可以耐强酸、 强碱。
请参看图 1 、 7所示， 若鞋材本体 10为鞋垫 100或鞋底 102， 为了提高鞋垫 100或鞋底 102的强度， 可在鞋垫 100或鞋底 102上局部位置加设复数个补强体 15， 借以提升鞋垫 100或鞋底 102的支撑性及回弹性， 该补强体 15的材料可为 聚氨酯 （PU, Polyurethane) , 热塑性弹性体 (TPE, Thermoplastic Elastomer) 或 EPA , 使其效果更为彰显更增加耐用度， 其制法系直接将聚氨酯 （PU, Polyurethane), 热塑性弹性体 (TPE, Thermoplastic Elastomer)或 EPA材料灌注到 鞋垫 100或鞋底 102， 经干燥后， 即可在鞋垫 100或鞋底 102上形成补强体 15。
本发明的鞋材本体 10可以为鞋底 102(如图 7所示)或鞋垫 100 (如图 1、 图 2 所示） ， 亦可以是鞋面 101(如图 3所示)， 其中， 鞋垫 100是供置入鞋子 20内以 间隔鞋底与人的脚底， 借以产生缓冲气垫作用及避免鞋底快速磨损。 其中， 该鞋 材本体 10为鞋垫 100， 该鞋垫 100包括该周边轮廓区域 1 1、 该内围区域 12及该 网体 120。 其中， 该鞋垫 100的该周边轮廓区域 1 1可为一胶剂层， 以该胶剂层固 定该纤维 13末端。 再者， 该鞋材为鞋垫 100， 该鞋垫 100的该周边轮廓区域 1 1 亦可为一由网体 120的该纤维 13相互热融黏合的熔结线 1 10， 以该熔结线 1 10 固定该纤维 13末端。
再者， 请参看图 5、 图 7所示， 本发明的鞋材本体 10为鞋底 102或鞋垫 100 时， 其可包括有复数层编织网体 120， 借以使内围区域 12的厚度增加， 以增加透 气性及缓冲气垫效能， 其每一网体 120为包括有复数条经向纤维 13及复数条纬 向纤维 13的网状编织体， 而各层的周边轮廓区域 1 1为一由该纤维 13 自体相互 粘合的熔结线 1 10， 以该熔结线 1 10固定该纤维 13末端。 如图 5所示， 其中， 本 发明一种较佳实施例， 该内围区域 12具有至少一个呈点状粘结部或线段状的粘 结部 121， 该粘结部 121为一由该网体 120的该纤维 13 自体相互粘结而成，借以 提高各网体 120之间相互叠合的牢固性。
又请参看图 6所示， 本发明的鞋材本体 10为鞋垫 100， 则又可设计成更包 括有至少一布层 14， 该布层 14覆设在该鞋垫 100的网体 120上， 而且该布层 14 的摩擦系数高于该网体 120的摩擦系数。 其中， 本发明一种较佳实施例， 该布层 14与该鞋垫 100的该网体 120之间以至少一个呈点状或线段状的粘合部 140相粘 合， 借以提高网体 120与布层 14之间相互贴合的牢固性。
请参看图 7所示， 本发明的鞋材本体 10为鞋底 102时， 该鞋底 102连接有 弧形并可套在人体脚部的套带 103而构成拖鞋的结构形态。
请参看图 8-10所示， 其中， 本发明鞋材本体的网体 120， 系编织成包括有复 数个呈阵列的立体蜂巢结构 121， 每一该蜂巢结构 121系由复数条该经向纤维 13 沿着一第一凹弧面 122排列及复数条该纬向纤维 13沿着一第二凹弧面 123排列 所构成， 其中， 该第一凹弧面 122与该第二凹弧面 123相互交叉。 通过该立体蜂 巢结构 121的设计， 以提高鞋材的高结构强度及透气与缓冲气垫效果。
其中， 本发明纤维的第一种具体实施例， 该机能性微粒可为次微米电气石， 借以使鞋材具有产生负离子、 远红外线、 自净、 除臭、 抗静电、 防电磁波等功效 并可加入奈米竹炭、 氧化锌、 氧化铜、 氧化铁、 氧化硅、 氧化钨、 氧化锰、 氧化 钴及氧化镍之中至少一种的微粒健康因数。
本发明第二种具体实施例， 该机能性微粒亦可为奈米银粒子， 借以使鞋材具 有杀菌、 抗菌、 防霉、 防螨等健康功能， 且可加入甲壳素、 酵素或奈米贵金属铜、 锌、 金、 铂、 钯、 铌等之中至少一种的健康微粒杀菌、 抗菌、 防霉因数。
本发明第三种具体实施例， 该机能性微粒可为微胶囊， 该微胶囊内部设有一 容纳空间， 该容纳空间填设有一层各类的机能性材料， 而微胶囊壳材的材料可为 几丁聚醣、 热可塑弹性体等， 而该层机能性材料可为天然精油而使鞋材具有持久 芳香精油的机能， 并可搭配熏衣草、 柠檬、 桧木、 迷迭香、 尤佳利、 茶树、 檀香、 佛手柑、 松、 茉莉、 玫瑰、 洋甘菊、 依兰、 罗勒、 天竺葵、 白千层、 豆蔻、 麝香、 没药、 肉桂、 茴香、 乳香、 桔、 薄荷、 雪松、 广藿香、 玫瑰草、 丁香、 葡萄袖、 安息香、 姜、 香茅及马郁兰之中至少一种的天然精油。
通过上述机能性微粒材料的结合及材料结构特性，而研发出机能性健康养生 自净微尘鞋材。 可因应不同需求， 而设计出不同的鞋材机能及结构。
Π .本发明鞋材的制造方法
请配合参看图 11所示， 本发明制造如上述的鞋材的方法， 系采用至少一片 状的网体 120， 该网体 120为一包括有复数条经向纤维 13及复数条纬向纤维 13 的网状编织体， 而且该纤维 13 内混含有复数个机能性微粒 130(请配合参看图 4 所示)， 再以超音波加工法而使该网体 120上布设有至少一条由该纤维 13相互熔 结而成的熔结线 110(请参看图 12所示)， 以该熔结线 110为周边轮廓区 11， 并以 该周边轮廓区 11将该网体 120区隔出一内围区域 12，以该内围区域 12做为鞋材 本体 10的形状。
请参看图 11、 12所示， 本发明一种具体实施例中， 该超音波加工法系使用 包括一超音波产生装置 33， 一上模 30， 及一第一下模 31， 将该至少一网体 120 先置于该上模 30与该第一下模 31之间， 将该上模 30与该第一下模 31合模， 由 该超音波产生装置 33而使该上模 30产生超音波振动， 再由该超音波而使该网体 120上布设有至少一条由该纤维 13相互熔结而成的熔结线 110， 以该熔结线 110 为周边轮廓区域 11而将该至少一网体 120区隔出至少一该内围区域 12， 再以一 裁切方法沿着该熔结线 110裁切， 进而完成该鞋材的制造。
请配合参看图 5、 11所示， 本发明一种具体实施例中， 该第一下模 31加设 有至少一个呈点状或线段状的凸部 310， 而且该至少一网体 120为相迭合的复数 个网体 120，通过该凸部 310而使该复数个网体 120的该内围区域 12形成点状或 线段状的粘结部 121，该粘结部 121为一由该复数个网体 120的该纤维 13相互粘 结而成。
请参看图 13、 14所示， 本发明一种具体实施例中， 该裁切方法， 可再加设 一第二下模 32，该第二下模 32上设有与该熔结线 110的轮廓形状相似的切刀 320， 将该网体 120置于该上模 30与该第二下模 32之间， 将该上模 30与该第二下模 32合模， 由该超音波产生装置 33而使该上模 30产生超音波振动， 再由该第二下 模 32的该切刀 320沿着该熔结线 110切断。
III .本发明机能功效的验证
(i)本发明鞋材的机械性试验
Figure imgf000007_0001
保有要求的强度。
(ii)本发明鞋材的抗张强度:
表 2: 鞋材抗张强度 （kgf/cm2 )
未添加织物 电气石含量 1 % 电气石含量 2 % 电气石含量 3 % 电气石含量 4 % 电气石含量 5 %
1 21.886 23.728 22.765 21.345 22.706 22.086
2 23.725 19.174 21.129 22.349 20.609 20.308
3 26.816 24.627 21.764 22.047 21.086 21.117
4 21.314 18.032 21.796 19.449 21.625 20.598 5 22.108 24.499 22.229 23.603 21.855 21.717 平均值 23.1698 22.012 21.9366 21.7586 21.5762 21.1652 由表 2得知， 本发明鞋材的抗张强度也随着电气石含量增加而减少， 在电气 石含量 1 %时经向抗张强度下降约 5 %，在电气石含量 5 %时经向抗张强度下降约 8.6% , 但仍然保持相当高的抗张强度。
(iii) 水洗牢度试验：
表 3 : 鞋材水洗牢度 （Ion/cc )
Figure imgf000008_0001
如表 3，测试时条件为湿度 58 %、温度 29°C，测试前后仍维持良好的坚牢度， 负离子的产生量并未因水洗而减少。
(iv)本发明鞋材的远红外线效能试验
依红外线放射仪、 热电偶试验， 由表 4结果发现本发明鞋材有长久有远红外 线效能能力。
表 4
Figure imgf000008_0002
(V)本发明鞋材的除臭效能试验
分别以本发明鞋材， 采用 GC-MS依 JEM 1467测试法对于测量氨气 （NH3) 及乙醛 （CH3CHO ) 的浓度， 再测试醋酸 （CH3COOH) 的浓度的消除效能而得 下表的结果。 由表 5发现本发明鞋材具有较佳的除臭效能。
表 5 : 本发明鞋材， 依 JEM 1467测试法测所达的除臭结果
Figure imgf000008_0003
(vi)本发明鞋材的抗菌效能试验
表 6
0 Initial
Contaxt Time作用
测试菌种 Inoculation(CFU/ml) Redruction抗菌效果 (％)
1小时 （lhr later) 1小时（lhr later)
0小时接菌量
金黄色葡萄球菌 1.0 X 10' 3.0 x 104 99.9(%) 大肠杆菌 2.1 X 10' 1.6 x 103 99.9(%) 肺炎杆菌 7.3 X 105 3.0 x 104 95.9(%)
Figure imgf000009_0001
由表 6得知以 ASTM E 2149-01试验法， 本发明具有较佳的抗菌效能。 由表 7得知以 AATCC 147试验法， 本发明也具有较佳的抗菌效能。
( vii)本发明鞋材的防霉效能试验
表 8
Figure imgf000009_0002
由表 8得知以 AATCC 30 PAPT III、 JIS Z 2911 、 G21-96试验法， 本发明 具有较佳的防霉效能。
(viii)本发明鞋材的防尘螨效能试验
依日本尘螨加工制品协议会忌避效果评估试验-邱入阻止法， 如表 10发现本 鞋材有长久有防尘螨效能能力。
表 10
Figure imgf000009_0003
(ix) 本发明鞋材的芳香持久效能试验
由表 11的结果显示， 本发明历经三个月仍具有有效的芳香效果。
表 11
Figure imgf000009_0004
(X) 本发明鞋材纤维的芳香成分分析试验
由 GC-MS测试本鞋材纤维内含有天然精油成分而得下表的结果。 由表 12发现本鞋材能有效含有天然精油成分清净能力。
7 表 12
Figure imgf000010_0001
(xi)本发明鞋材的室内空气质量效能试验如下表：
依 JEM 1467测试法针对于测量室内空气质量 (IAQ)的消除效能而得表 13的 结果。 由下表 13发现本发明空气质量 (IAQ)长久有效自动清净能力。
表 13
Figure imgf000010_0002
(xii) 本发明鞋材的抗静电效能试验
依据 AATCC D4935-1999, 由表 14发现本鞋材有良好有抗电磁波效能能力。
表 14
试验项目 试验结果
织物表面电阻（ Ω /square) >E+11 (Xiii) 本发明鞋材的抗电磁波效能试验如下表：
依据 AATCC 756-1995 (试验条件为温度 20°C、 湿度 40%RH)， 由表 15发现 本鞋材有良好有抗静电效能能力。
表 15
Figure imgf000011_0001
(Xiv)本发明鞋材的低压损效能试验
依据美国冷冻空调协会 AHRAS 52.2 测试， 由表 16发现本发明有良好有低 压损能力。
表 16
Figure imgf000011_0002
(XV) 本发明鞋材的防火效能试验
依 UL 94-97方法， 由表 17发现本鞋材有长久有防火能力 VTM-0
表 17
Figure imgf000011_0003
(xvi)本发明鞋材的符合 RoHS环保效能试验
依样品所化验的化学物质一铅、 镉、 汞、 六价铬、 多溴联苯及多溴联苯醚的 测试结果， 符合 RoHS指令 (2002/95/EC)欧盟环保规范方法， 由表 18、 表 19发现 本鞋材有符合 RoHS规范。
表 18
Figure imgf000012_0001
表 19
测试项目 单位 测试方法 方法侦测 ROHS 限 极限值 NO.l
六价袼 mg/kg(pp 参考 US EPA 3060A方法， 2 N.D. 1000 m) 用 UV-VIS ( US EPA
7196A) 分析
镉 mg/kg(pp 参考 EN1122方法 B 2001 2 N.D. 100 m) 用感应耦合电浆原子发射
光谱仪 （ICP-AES ) 分析
汞 mg/kg(pp 参考 US EPA 3052方法， 2 N.D. 1000 m) 用感应耦合电浆原子发射
光谱仪 （ICP-AES ) 分析
铅 mg/kg(pp 参考 US EPA 3050方法， 2 N.D. 1000 m) 用感应耦合电浆原子发射
光谱仪 （ICP-AES ) 分析 IV. 结论
因此， 通过上述的结构设计， 可归纳本发明确实具有下列几点优点与特点：
1 .本发明鞋材的纤维内混含有机能性微粒，使鞋材具有产生机能性如杀菌、 抗菌、 防霉、 防螨、 负离子、 远红外线、 防火、 抗静电、 抗电磁波及排除异味、 TVOCs、 PMx等污染物等健康养生的功效。
2 . 本发明鞋材为鞋垫而具有多层结构， 使纤维在兼顾机械性质的原则下而 具有较佳的弹性， 让流体经过鞋材时， 能产生适当的振动效能， 激使纤维内的机 能性微粒更为活泼作用， 而达到有效发挥其健康机能的效果并能使足部得到适当 纡缓及运动缓冲的机能性气垫
3 . 本发明鞋材为鞋垫， 其以纤维编织， 具较佳通风， 可确实达成卫生及健 康的功效及可水洗。
4 . 本发明鞋材添加机能性微粒 （如次微米电气石粒子） ， 其所制成的鞋材 的机械强度， 仅些微的减低， 但无太大影响。
5 . 本发明鞋材添加机能性微粒（如次微米电气石粒子）， 经水洗牢度试验， 仍保有一定的功能。
6 . 本发明次微米电气石粒子， 因电气石带负电效果， 在 「静电吸附原理」 下而能有效增加提升效能， 鞋材不仅具有较佳弹性、 摩擦性， 由于负离子特殊功 效-热电性、 压电性加速水分解负离子 （H3O2— ) 下， 弹性振动频率高， 摩擦力较 大， 动态模式下便可大量释放出负离子量， 而能确实符合人体健康的需求量 (1000-2000ion/cc)o
7 . 本发明添加包含有精油的微胶囊时， 避免精油快速挥发， 而可使精油以 接近定量的方式释出， 避免浪费及增进耐久性。
8 .本发明鞋材添加奈米银粒子时，使得本发明的鞋材具有一定的抗菌效果。 9 . 本发明的鞋材也具有防火的功能， 可以确保使用上绝对的防火安全性。

Claims

权 利 要 求
1.一种多功能机能性健康养生自净鞋材， 其包括：
一鞋材本体， 该本体包括有周边轮廓区域及内围区域； 以及
至少一个分布在该本体的该内围区域的片状网体，该网体被固定在该周边轮 廓区上， 该网体为包括有复数条经向纤维及复数条纬向纤维的网状编织体， 而且 该纤维内包含有复数个机能性微粒。
2.如权利要求 1所述的多功能机能性健康养生自净鞋材， 其中， 该本体的该 内围区域是由复数片的网体所叠合而成。
3.如权利要求 2所述的多功能机能性健康养生自净鞋材， 其中， 该内围区域 具有至少一个呈点状或线段状的粘结部， 该粘结部为一由该复数片网体的该纤维 相互粘结而成。
4.如权利要求 1所述的多功能机能性健康养生自净鞋材， 其中， 该鞋材本体 为鞋面。
5.如权利要求 1所述的多功能机能性健康养生自净鞋材， 其中， 该鞋材本体 为鞋垫， 该鞋垫包括有该周边轮廓区域、 该内围区域及该网体。
6.如权利要求 5所述的多功能机能性健康养生自净鞋材， 其更包括有至少一 布层， 该布层覆设在该鞋垫的该网体上， 该布层的摩擦系数高于该网体的摩擦系 数。
7.如权利要求 6所述的多功能机能性健康养生自净鞋材， 其中， 该布层与该 鞋垫的该网体之间以至少一个呈点状或线段状的粘合部相粘合。
8.如权利要求 5所述的多功能机能性健康养生自净鞋材， 其中， 该鞋垫的该 周边轮廓区域为一由该纤维自体相互粘结的粘结层， 以该粘结层固定该纤维末
4 9.如权利要求 1所述的多功能机能性健康养生自净鞋材， 其中， 该鞋材本体 的该网体编织成包括有复数个呈阵列的立体蜂巢结构， 每一该蜂巢结构系由复数 条该经向纤维沿着一第一凹弧面排列及复数条该纬向纤维沿着一第二凹弧面排 列所构成， 其中， 该第一凹弧面与该第二凹弧面相互交叉。
10.如权利要求 1 所述的多功能机能性健康养生自净鞋材， 其特征在于， 该 鞋材本体为鞋底， 该鞋底包括有该周边轮廓区域及该内围区域。
11.如权利要求 10的多功能机能性健康养生自净鞋材， 其中， 该鞋底连接有 弧形并可套在人体脚部的套带而构成拖鞋的结构形态。
12.如权利要求 1 的多功能机能性健康养生自净鞋材， 其中， 该鞋材本体为 一鞋垫或一鞋底， 该鞋垫或该鞋底上局部位置以灌注方式而加设复数个补强体。
13.如权利要求 12的多功能机能性健康养生自净鞋材， 其中， 该补强体的材 料系选自 PU、 TPE及 EPA至少其中一种。
14.如权利要求 1 的多功能机能性健康养生自净鞋材， 其中， 该纤维的线径 可介于 50-10000丹尼之间。
15.如权利要求 1 所述的多功能机能性健康养生自净鞋材， 其中， 该机能性 微粒系选自包括有次微米电气石、 二氧化钛、 奈米竹炭、 氧化锌、 氧化铜、 氧化 铁、 氧化硅、 氧化钨、 氧化锰、 氧化钴、 氧化镍、 奈米银粒子、 甲壳素、 酵素或 奈米贵金属铜、 锌、 金、 铂、 钯、 铌、 微胶囊、 酵素及光触媒中至少一种微粒因 数。
16.如权利要求 15的多功能机能性健康养生自净鞋材， 其中， 该微胶囊内部 具有容纳空间， 该容纳空间填设有一层天然植物萃取精油， 该层植物萃取精油系 选自包括熏衣草、 柠檬、 桧木、 迷迭香、 尤佳利、 茶树、 檀香、 佛手柑、 松、 茉 莉、 玫瑰、 洋甘菊、 依兰、 罗勒、 天竺葵、 白千层、 豆蔻、 麝香、 没药、 肉桂、 茴香、 乳香、 桔、 薄荷、 雪松、 广藿香、 玫瑰草、 丁香、 葡萄袖、 安息香、 姜、 香茅及马郁兰中至少一种天然精油。
17.—种鞋材的制造方法， 该鞋材本体包括有周边轮廓区域、 内围区域及至 少一个分布在该本体的该内围区域的片状网体， 该网体被固定在该周边轮廓区 上， 该网体为包括有复数条经向纤维及复数条纬向纤维的网状编织体， 而且该纤 维内混含有复数个机能性微粒， 该制造方法包括， 系采用至少一片状的该网体， 再以超音波加工法而使该网体上布设有至少一条由该纤维相互熔结而成的熔结 线， 以该熔结线为该周边轮廓区， 并以该周边轮廓区将该网体区隔出一该内围区 域， 以该内围区域做为该鞋材本体的形状。
18.如权利要求 17所述的制造方法， 其中， 该超音波加工法系使用包括一超 音波产生装置， 一上模， 及一第一下模， 将该至少一网体先置于该上模与该第一 下模之间， 将该上模与该第一下模合模， 通过该超音波产生装置而使该上模产生 超音波振动， 再通过该超音波而使该网体上布设有至少一条由该纤维相互熔结而 成的熔结线， 并使该熔结线将该至少一网体区隔出至少一该内围区域， 再以一裁 切方法沿着该熔结线裁切， 进而完成该鞋材的制造。
19.如权利要求 18所述的制造方法， 其中， 该第一下模加设有至少一个呈点 状或线段状的凸部， 而且该至少一网体为相迭合的复数个网体， 由该凸部而使该 复数个网体的该内围区域形成点状或线段状的粘结部， 该粘结部为一由该复数个 网体的该该纤维相互粘结而成。
20.如权利要求 18所述的制造方法， 其中， 该裁切方法， 可再加设一第二下 模， 该第二下模上设有与该熔结线的轮廓形状相似的切刀， 将该网体置于该上模 与该第二下模之间， 将该上模与该第二下模合模， 通过该超音波产生装置而使该 上模产生超音波振动， 再通过该第二下模的该切刀沿着该熔结线切断。
21.如权利要求 17所述的制造方法， 其中， 该鞋材系选自鞋面、 鞋垫及鞋底 ^ ψ——禾中。
22.如权利要求 17所述的制造方法， 其中， 该机能性微粒系选自包括有次微 米电气石、 二氧化钛、 奈米竹炭、 氧化锌、 氧化铜、 氧化铁、 氧化硅、 氧化钨、 氧化锰、 氧化钴、 氧化镍、 奈米银粒子、 甲壳素、 酵素或奈米贵金属铜、 锌、 金、 铂、 钯、 铌、 微胶囊、 酵素及光触媒中至少一种微粒因数。
23.如权利要求 22的多功能机能性健康养生自净鞋材， 其中， 该微胶囊内部 具有容纳空间， 该容纳空间填设有一层天然植物萃取精油， 该层植物萃取精油系 选自包括熏衣草、 柠檬、 桧木、 迷迭香、 尤佳利、 茶树、 檀香、 佛手柑、 松、 茉 莉、 玫瑰、 洋甘菊、 依兰、 罗勒、 天竺葵、 白千层、 豆蔻、 麝香、 没药、 肉桂、 茴香、 乳香、 桔、 薄荷、 雪松、 广藿香、 玫瑰草、 丁香、 葡萄袖、 安息香、 姜、 香茅及马郁兰中至少一种天然精油。
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NZ579521A NZ579521A (en) 2007-03-12 2008-03-11 Shoe insert including inner web with functional particles
JP2009552995A JP2010520792A (ja) 2007-03-12 2008-03-11 多功能、機能性の健康養生及びセルフ−クリーン効果を有する靴素材
AU2008226237A AU2008226237B2 (en) 2007-03-12 2008-03-11 Multi-function health care self-cleaning shoe material
US12/449,891 US20100050469A1 (en) 2007-03-12 2008-03-11 Multi-function health care self-cleaning shoe material
EP08715200A EP2130448A4 (en) 2007-03-12 2008-03-11 SELF-CLEANING HEALTH PROTECTION SHOE MATERIAL WITH MULTIFUNCTION
MX2009009275A MX2009009275A (es) 2007-03-12 2008-03-11 Material multi-funcional para autolimpiado del zapato para el cuidado de la salud.
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CN201039770Y (zh) 2008-03-26
EP2130448A1 (en) 2009-12-09
CA2682318A1 (en) 2008-09-18
JP2010520792A (ja) 2010-06-17
EP2130448A4 (en) 2013-02-27
AU2008226237B2 (en) 2013-03-14
AU2008226237A1 (en) 2008-09-18
MX2009009275A (es) 2010-03-22
US20100050469A1 (en) 2010-03-04
NZ579521A (en) 2012-04-27

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